Szczegóły publikacji
Opis bibliograficzny
A parametric analysis of the long term performance of a solid oxide fuel cell anode / Tomasz A. PROKOP, Szymon BUCHANIEC, Janusz SZMYD, Grzegorz BRUS // International Journal of Heat and Fluid Flow ; ISSN 0142-727X. — 2024 — vol. 110 art. no. 109583, s. 1–8. — Bibliogr. s. 7–8, Abstr. — Publikacja dostępna online od: 2024-09-26
Autorzy (4)
Słowa kluczowe
Dane bibliometryczne
| ID BaDAP | 155676 |
|---|---|
| Data dodania do BaDAP | 2024-10-28 |
| Tekst źródłowy | URL |
| DOI | 10.1016/j.ijheatfluidflow.2024.109583 |
| Rok publikacji | 2024 |
| Typ publikacji | artykuł w czasopiśmie |
| Otwarty dostęp | |
| Creative Commons | |
| Czasopismo/seria | International Journal of Heat and Fluid Flow |
Abstract
Solid oxide fuel cells are a type of a fuel cell characterized by exceptional efficiency and flexibility. Previous experimental studies have shown that, while the fine particle radius in the nickel-YSZ cermet of the anode corresponds to greater availability of reaction sites, it also causes an increased rate of microstructure degradation. However, long-term performance issues continue to hinder their widespread implementation. In this study a parametric analysis is performed in order inspect the relationship between the initial grain radia in the microstructure and its long-term performance. Anodic microstructures in their initial state are artificially generated using cellular automata methodology. Then, long-term degradation is simulated using a phase field model combined with an electrochemical performance model in order to predict the voltage output of a particular anode design. The long-term degradation model has been previously validated through comparison to a real life, 3800 hour-long performance test. The simulations include 6 000 hour-long period during which higher than expected durability was predicted for microstructures with high initial reaction site density. The results can be applied in smart electrode design and optimization.